I have been getting this problem randomly and never know the reasons. Today I got bad holes again.
If it's random...... It's not something that is unchanging... I wouldn't jump to the tool first.
1) 3 mm 120 deg carbide spot drill, 4.2 mm 130 deg M42 HSS drill, good holes on 6061 and 7075 aluminum, no chattering
2) same as above but the material of the workpiece is mild steel, some chattering, bad holes as shown in the photo. Have tried 6 holes, all bad.
I question this here. Using a 120 spot drill for a "larger than 120" drill bit forces it to start it's cut on the corners. At 4.2mm (five thirty twos, or number 19,20 ish in the wire gauge drills for inch folks reading), the drill isn't that rigid. When it starts on the two outer flutes, it's gonna wobble, and it isn't rigid enough to recover from that.
When you choose different materials, different RPMs, different feed rates (or feed pressure), it WILL change that characteristeric, for better or for worse. How you "hit" the spot drill mark can also make a difference. Ease in and let it "bore" it's own center while you hope it still guides some, (usually better on smaller drills, but being a touchy feely intuition thing.... Anything goes). Or the "plow through it quick and get the center of the drill to the center of the spot as fast as you can appoach. (usually better on larger drills, but again, anything goes).
So those are my thoughts. I wouldn't say I know the answer, as I havn't seen in person or used your drill. But if it's random, it's "probably" something you are doing, vs the drill being good or bad from day to day. Or your spindle bearings loosening and tightening from day to day. The spot drill at the wrong angle WILL aggrivate that situation. (Although it often works... I'm as guilty as anybody).
3) 6 mm 120 deg carbide spot drill, 6 mm 130 deg M35 HSS drill, good holes on all materials mentioned above. No chattering
Oil used in all cases.
What might be the reasons ? Is the 4.2 mm drill to be blamed ? It's new.
The 6mm drill bit (15/64 ish, or number A,B ish in wire gauge) is a much more robust drill, with (roughly) twice as much cross sectional area. You can get away with a lot more. They're both still small, it's not a free for all with either, but you can get away with more.
Were it me, having this issue, I'd validate my suspicion (again, that's all it is), by taking the 4.2mm drill, with no spot drill, perhaps a center pop just large enough to capture the split point, but no more, and I'd just plow. By that I mean not "how strong are you", or "how fast is your power feed", but bear down until it makes a good continuous chip, and keep up with it. Keep that chip as long as you can keep it. Then examine the hole. If that solves the problem, you have a solution. Fix the spot drill thing. If that does nothing, it's gotta be something else, right? What else has changed from "good holes" to "poor holes"? Even if my first thought is wrong, I still say that. If it's random, and "sometimes" that the problem occurs.... It's a variable that's changing in between uses.