Heating chromium has the potential to generate chromium in the hexavalent state, a very toxic substance. Wikipedia has
some good information on Chromium6 (hexavalent chromium). I have no idea what chemistry might be involved with heating
brass and chromium but I do know that under the right conditions, chromium can do serious damage to the body.
I would tend to err on the careful side with a mix of copper, zinc, and chromium heated to 1800F and at a very minimum
would do this outside and stay upwind of the crucible and better yet not use the chrome plated brass.